C K-edge inner-shell spectra of liquid alcohols obtained from the snapshots of molecular dynamics simulations

For reproducing C K-edge XAS spectra of liquid alcohols such as ethanol and methanol, the inner-shell calculations were performed with the snapshots of the liquid structures obtained by molecular dynamics simulations. The C K-edge inner-shell spectrum of liquid ethanol was obtained by the summation of one thousand calculated spectra including neighbor molecules within the CH2‒CH2 distance of 6 Å. The calculated C K-edge inner-shell spectra of liquid alcohols well reproduced the spectral shapes of the experimentally obtained XAS spectra and the spectral changes from gas to liquid phases.

  1. M. Nagasaka, J. Chem. Phys. 158, 024501 (2023).